Using ultrafast nonlinear-optical response of organic dye films, a train of picosecond optical pulses can be converted into a space pattern of a mm scale. As applications of this technique we demonstrate a single-shot multichannel optical switching for 1 Tbit/s pulse trains, and a timing jitter suppression of pulse trains using a control system with femtoseconds time resolution.

We fabricated ultrafast nonlinear optical films of squarylium J-aggregates and studied their properties including the absorption spectrum, the refractive index, the third-order nonlinear optical coefficients, the extent of absorption saturation, and the recovery of absorption saturation. The transmittance of the film was increased by 30% due to absorption saturation at a pump energy of several hundreds fJ/µm2/pulse. The half decay time constant of absorption saturation was found to be approximately 100 fs for off-resonant excitation. Two-dimensional demultiplexing was demonstrated using the squarylium film as a switching material. From a train of 8 optical pulses with 100 fs duration and 1 ps interval corresponding to a bit rate of 1 Tbps, 24 spatially resolved spots were obained.