Codebooks with small maximal cross-correlation amplitudes have important applications in code division multiple access (CDMA) communication, coding theory and compressed sensing. In this letter, we design a new codebook based on a construction of Ramanujan graphs over finite abelian groups. We prove that the new codebook with length K=q+1 and size N=q2+2q+2 is asymptotically optimal with nearly achieving the Levenshtein bound when n=3, where q is a prime power. The parameters of the new codebook are new.